Character | How to unlock
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A.I.M. Agent | Complete Level 10: That Sinking Feeling.
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Abomination | Complete Level 4: Rock up at the Lock up.
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Absorbing Man | Collect his token in Industrial District.
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Agent Coulson | Complete Bonus Level: Tabloid Tidy UP.
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Aldrich Killian | Complete Level 5: Rebooted, Resuited.
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Ant-Man | Collect his token in the Industrial District.
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Archangel | Collect his token south of the X-Mansion, to the south of giant billboard.
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Arnim Zola | Complete Level 6: Red Head Detention.
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Aunt May | Complete Deadpool's 3 missions.
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Beast | Complete Level 8: Juggernauts and Crosses.
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Beetle | Collect his token a block east of the central park lake.
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Black Bolt | Complete Gambit's first mission.
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Black Cat | Collect her token below Lady Liberty on the map in a cat pet shop (requires Spider Man to unlock).
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Black Panther | Complete his 3 missions.
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Black Widow | Complete Level 3: Exploratory Laboratory.
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Blade | Complete his 3 missions.
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Blob | Complete Bonus Level: Put Up Your Dukes.
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Bullseye | Collect his token in Slums District.
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Captain America | Complete Level 2: Times Square Off.
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Captain America (Comics) | Complete Bonus Level: The Brick Apple.
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Captain Britain | Complete Bonus Level: The Brick Apple.
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Carnage | Collect his token in Residential District.
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Colossus | Collect Colossus token in the front right courtyard of the X-Mansion.
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Cyclops | Complete Level 8: Juggernauts and Crosses.
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Cyclops (Astonishing) | Taxi the character in the Financial District to his destination, then collect his token.
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Damage Control | Put the out fires on the SHIELD Helicarrier deck with the water gun.
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Daredevil | Complete Bonus Level: Feeling Frisky.
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Deadpool | Collect all Deadpool Red Bricks.
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Doctor Doom | Complete Level 14: "A Doom with a View".
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Doctor Octopus | Complete Level 2: Times Square Off.
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Doctor Octopus (Ultimate) | Complete Bonus Level: Tabloid Tidy UP.
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Doctor Strange | Complete Bonus Level: Stranger Danger.
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Doombot | Complete Level 9: Doctor in the House.
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Doombot (V-Series) | Complete Level 14: "A Doom with a View".
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Drax the Destroyer | Complete the story, then complete his 3 missions.
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Electro | Complete Bonus Level: A Shock Withdrawal.
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Electro (Ultimate) | Taxi the character in front of the Oscorp building to her destination, then collect his token.
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Elektra | Collect her token in Slums District.
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Emma Frost | Complete a mission Professor X hands out.
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Frost Giant | Complete Level 7 - Bifrosty Reception.
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Galactus (Minifig) | Complete Level 15: The Good, the Bad and the Hungry.
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Gambit | Complete his 3 missions.
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Gamora | Complete the story, then complete the first mission you get from Drax.
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Ghost Rider | Complete Bonus Level: Stunt Show Surprise.
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Green Goblin | Complete Level 9: Doctor in the House.
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Green Goblin (Ultimate) | Collect his token in Bonus Level: Thrill of the Chess.
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Groot | Complete the story, then complete his 3 missions.
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Gwen Stacy | Complete "Mission 47" for Drax.
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H.E.R.B.I.E. | Complete Level 2: Times Square Off.
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Havok | Collect his token in the Forest District.
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Hawkeye | Complete Level 3: Exploratory Laboratory.
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Heimdall | Complete his 3 missions.
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Howard the Duck | Complete Bonus Level: Nuff Said.
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Hulk | Complete Level 1: Sand Central Station.
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Human Torch | Complete Level 6: Red Head Detention.
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Hydra Agent | Collect his token in the Forest District.
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Iceman | Complete Level 8: Juggernauts and Crosses.
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Invisible Woman | Complete Level 9: Doctor in the House.
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Invisible Woman (Future Foundation) | Collect her token in Bonus Level: Stranger Danger.
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Iron Fist | Complete race mission with Blade, then win the fight with ice dudes in the next Blade mission.
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Iron Man (Heroic Age) | Complete Bonus Level: New York Event.
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Iron Man (Hulkbuster) | Land on "S" sign landing platform, then take out all the airvents that are all around the "S" sign.
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Iron Man MK I | Complete Level 5: Rebooted, Resuited.
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Iron Man MK VI | Complete Level 1: Sand Central Station.
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Iron Man MK VII | Complete Bonus Level: House Party Protocol.
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Iron Man MK XLVII | Complete Level 5: Rebooted, Resuited.
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Iron Man MK XVII | Complete Bonus Level: House Party Protocol.
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J. Jonah Jameson | Complete Bonus Level: Tabloid Tidy Up.
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Jean Grey | Complete Level 8: Juggernauts and Crosses.
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Juggernaut | Complete Level 8: Juggernauts and Crosses.
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Kingpin | Complete Bonus Level: Feeling Frisky.
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Kingpin Henchman | Collect his token in Bonus Level: Feeling Frisky.
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Kraven the Hunter | Shoot the five targets next to the Godzilla-looking icon at the Central Park.
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Kurse | Defeat him in battle near Roxxon Power Station, then collect his token.
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Lady Liberty (Minifig) | Complete Level 11: Taking Liberties.
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Laufey | Complete Bonus Level: Bro-tunheim.
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Loki | Complete Level 15: The Good, the Bad and the Hungry.
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M.O.D.O.K. | Complete Level 10 - That Sinking Feeling.
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Magneto | Complete Level 13 - Magnetic Personality.
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Magneto Acolyte | Complete Level 13: Magnetic Personality.
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Malekith | Complete Bonus Level: Bro-tunheim.
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Mandarin (Film) | Collect his token in Bonus Level: Stunt Show Surprise.
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Maria Hill | Complete her 3 missions on the Helicarrier.
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Mary Jane Watson | Collect her token in the Residential District.
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Mister Fantastic | Complete Level 2: Times Square Off.
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Mister Fantastic (Future Foundation) | Defeat Ghost Rider in a race starting in West Harlem.
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Moon Knight | Collect his token in Bonus Level: A Shock Withdrawl.
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Ms. Marvel | Collect her token in Bonus Level: 'Nuff Said.
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Mysterio | Complete Bonus Level: Thrill of the Chess.
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Mystique | Complete Level 12: Rapturous Rise.
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Nick Fury | Complete Level 9: Doctor in the House.
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Nightmare | Complete Bonus Level: Stunt Show Surprise.
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Nova | Complete foot race mission with him at the east of the giant Godzilla icon in the Central Park.
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Pepper Potts | Complete Black Panther's first mission.
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Phoenix | Complete Bonus Level: Put up your Dukes.
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Polaris | Complete Bonus Level: Thrill of the Chess.
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Power Man | Collect his token in Yorkville District.
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Professor Xavier | Complete his 3 missions behind the X-Mansion.
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Psylocke | Complete all Captain Britain missions.
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Punisher | Complete his 3 missions.
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Pyro | Complete Level 8: Juggernauts and Crosses.
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Red Hulk | Defeat Red Hulk in battle, then collect his token.
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Red Skull | Complete Level 6: Red Head Detention.
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Rescue | Complete Black Panther's second mission.
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Rhino | Complete Level 12: Rapturous Rise.
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Rocket Raccoon | Complete his 3 missions.
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Ronan the Accuser | Find hidden path behind the statue south of his icon.
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Roxxon Agent | Complete Level 1: Sand Central Station.
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S.H.I.E.L.D. Agent | Collect his token on the Helicarrier.
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Sabretooth | Complete Level 4: Rock Up at the Lock Up.
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Sandman | Complete Level 1: Sand Central Station.
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Sandman Goon | Collect his token directly east of the Lizard House near the water.
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Sentinal (Minifig) | Defeat the Sentinal, then collect its token.
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She-Hulk | Collect her token in the Scrapyard.
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Shocker | Complete Bonus Level: A Shock Withdrawl.
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Silver Samurai | Collect his token in the Industrial District.
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Silver Surfer | Complete his 3 missions.
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Spider-Man | Complete Level 1: Sand Central Station.
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Spider-Man (Future Foundation) | Defeat Ghost Rider in a race in the Dockyard.
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Spider-Woman | Collect her token west of the park on the southern most part of the island.
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Squirrel Girl | Collect her token in the Dockyard.
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Stan Lee | Rescue all 50 Stan Lee in Peril.
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Star-Lord | Complete his 3 missions.
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Storm | Complete Level 8: Juggernauts and Crosses.
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Super-Skrull | Collect his token in the Upper East Side.
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Superior Spider-Man | Skydive off the Empire State Building, falling through the rings of studs. You will collect this token near the ground.
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Symbiote Scientist | Complete Level 3: Exploratory Laboratory.
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Symbiote Scientist (Hazmat) | Complete Level 3: Exploratory Laboratory.
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Taskmaster | Collect his token on a platform above the clouds east of Liberty Island.
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The Destroyer (Minifig) | Complete Level 7: Bifrosty Reception.
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The Leader | Collect his Token near Fisk Tower.
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The Mandarin | Complete Level 5: Rebooted, Resuited.
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Thing | Complete Level 9: Doctor in the House.
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Thing (Future Foundation) | Collect his token in Bonus Level: Reptillian Ruckus.
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Thor | Complete Level 7: Bifrosty Reception.
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Thor (Classic) | Collect his token in Bonus Level: Bro-tunheim.
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Toad | Complete his 3 missions.
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Tony Stark | Complete Level 5: Rebooted, Resuited.
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Tony Stark (Underwear) | Complete Level 4: Rock up at the Lock up.
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Union Jack | Complete Bonus Level: The Brick Apple.
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Venom | Complete Level 3: Exploratory Laboratory.
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Viper | Collect his token in Central Park.
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Vulture | Complete Bonus Level: 'Nuff Said.
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War Machine | Complete Bonus Level: House Party Protocol.
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Wasp | Collect his token one block south of the Oscorp Building.
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Whiplash | Collect his token in Yorkville.
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Wizard | Collect his token on the Baxter Building.
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Wolverine | Complete Level 4: Rock up at the Lock up.
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Wolverine (Cowl) | Collect his token in Bonus Level: Put up your Dukes.
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